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Personally - I think e-mail is the perfect first contact. It can be recieved and responded to quickly.
If one party doesn't have e-mail, then I'd say letter.
That way you can get out all your feelings - no awkward pauses, and you can read it over and over to reflect on everything. In a phone call, so many things may be said, you can't possibly remember it all.
Maybe start out with a letter, then agree on a good time for a phone call.
Best of luck and congrats!
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